Direct structural evidence of commensurate-to-incommensurate transition of hydrocarbon adsorption in a microporous metal organic framework

نویسندگان

  • Debasis Banerjee
  • Hao Wang
  • Qihan Gong
  • Anna M. Plonka
  • Jacek Jagiello
  • Haohan Wu
  • William R. Woerner
  • Thomas J. Emge
  • David H. Olson
  • John B. Parise
  • Jing Li
چکیده

Department of Chemistry and Chemical Bi 08854, USA. E-mail: [email protected] Department of Geosciences, Stony Brook Un Micromeritics Instrument Corporation, 435 30093, USA † Electronic supplementary information ( gas-adsorption data and crystallographic and 1427863. For ESI and crystallographic see DOI: 10.1039/c5sc03685b ‡ These authors contributed equally to th Cite this: Chem. Sci., 2016, 7, 759

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Study of the dynamic adsorption process of toluene by a microporous copper metal-organic framework

Introduction: Toluene is considered as a group of chemical contaminants, causing problems for people’s health. Due to the high rate of evaporation and rapid emission in the surrounding environment, it leads to the exposure of many employees and people at risk and, subsequently, its irreparable effects on their health in different jobs. Therefore, its removal is very important. In the present st...

متن کامل

Hydrogen storage in metal–organic frameworksw

New materials capable of storing hydrogen at high gravimetric and volumetric densities are required if hydrogen is to be widely employed as a clean alternative to hydrocarbon fuels in cars and other mobile applications. With exceptionally high surface areas and chemically-tunable structures, microporous metal–organic frameworks have recently emerged as some of the most promising candidate mater...

متن کامل

Optimization of solvothermally synthesized ZIF-67 metal organic framework and its application for Cr(VI) adsorption from aqueous solution

In this study, ZIF-67 was synthesized through solvothermal method to remove Cr(VI) ions from aqueous solution. To improve the structural properties of ZIF-67 and its adsorption capacity, optimization of the synthesis conditions was carried out based on maximum Cr(VI) uptake. From experiments, the optimum condition was revealed as solvent: metal ion molar ratio of 4.6:1, ligand: metal ion molar ...

متن کامل

Efficient removal of cobalt(II) ion from aqueous solution using amide-functionalized metal-organic framework

In this study, an amide-functionalized metal-organic framework, namely TMU-24 was selected to adsorb Co(II) from wastewater with an adsorption capacity of 500 mg. g-1 in less than 20 minutes in neutral pH (pH=7). The effect of diverse parameters such as adsorbent dosage, competitive ions, and contact time on the adsorption process was investigated to find the optimal amounts of them. Also, the ...

متن کامل

An Experimental Study of Adsorption Breakthrough Curves for CO2/CH4 Separation in a Fixed Bed of Nanoporous Shaped Copper Trimesate Metal Organic Framework

Copper trimesate (Cu-BTC) MOF has been pointed out as a promising adsorbent for separating carbon dioxide from methane. However, MOF’s need to be shaped prior to their use in packed bed adsorbers in order to reduce pressure drop; on the other hand, the production of mechanically resistant shaped bodies reduces their adsorption performance. In this work, Cu-BTC tablets provided by BASF are evalu...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2015